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Foreword ( Research on Chemical Intermediates , Volume 27 , Issue 1-2 )

Irradiation-dependent equilibrium between open and closed form of UV absorbers of the 2-(2-hydroxyphenyl)-1,3,5-triazine type

Optical and electrochemical cations recognition and release from N-azacrown carbazoles

Molecular dynamics simulation of the geminate radical recombination in solution: effects of the large dipole moment of the radicals

Benzylbenzoin benzyl ethers as new photoinitiators

A reduction of the high symmetry of C$_{60}$ in a PMMA polymer film as revealed by electroabsorption spectra

Pico- and nano-second laser flash photolysis study on photoinduced charge separation in oligothiophene-C$_{60}$ dyad molecules

Effect of ion-exchanged alkali metal cations on the photolysis of 2-pentanone included within ZSM-5 zeolite cavities: a study of ab initio molecular orbital calculations

Theory of electron transfer reactions in blue-copper proteins

Excited state dynamics of Michler's ketone: a laser flash photolysis study

Photochemical reaction intermediates of benzyl chloride in condensed phase

Magnetic field effects on the triplet exciplex dynamics in the duroquinone-N,N-dimethylaniline derivative systems

Intermolecular complexes between sulfide radical cations from β-hydroxy sulfides and phosphate

Direct observation of interfacial hole transfer from a photoexcited TiO$_{2}$ particle to an adsorbed molecule SCN$^{-}$ by femtosecond diffuse reflectance spectroscopy

Studies on reactivity of benzoyl and benzoylperoxy radicals produced by laser flash photolysis of dibenzoyldiazene in aerated solutions

Water-induced fluorescence quenching of aniline and its derivatives in aqueous solution

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Intermolecular complexes between sulfide radical cations from β-hydroxy sulfides and phosphate

Content Provider	Springer Nature Link
Author	Schöneich, Christian Miller, Brian Hug, Gordon L. Bobrowski, Krzysztof Marciniak, Bronislaw
Copyright Year	2001
Abstract	Triplet-sensitized oxidation of 2-(methylthio)ethanol (2-MTE) and photosensitized formaldehyde formation from 2-MTE were measured in aqueous solutions. The formaldehyde quantum yields were measured in steady-state experiments; whereas the time-resolved detection of dimeric sulfur radical cations (S∴S)$^{+}$ was followed in nanosecond laser flash photolysis. 4-Carboxybenzophenone was the triplet sensitizer in both types of experiments. It was found that the lifetimes of the (S∴S)$^{+}$ radicals increased in the presence of phosphate buffer, sodium perchlorate, or D$_{2}$O. There were corresponding decreases in the formaldehyde yields for these same experimental factors. The phosphate case was discussed in some detail in terms of a new intermolecular complex between the sulfide radical cations and the oxyanions.
Starting Page	165
Ending Page	175
Page Count	11
File Format	PDF
ISSN	09226168
Journal	Research on Chemical Intermediates
Volume Number	27
Issue Number	1-2
e-ISSN	15685675
Language	English
Publisher	Brill Academic Publishers
Publisher Date	2001-01-01
Publisher Place	Leiden
Access Restriction	One Nation One Subscription (ONOS)
Subject Keyword	Inorganic Chemistry Physical Chemistry
Content Type	Text
Resource Type	Article
Subject	Chemistry

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Ionization potentials of non-metal monosulfides. Conjugation in radical cations containing Group IV elements

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Inclusion complexation of N-substituted phenothiazines and their radical cations generated electrochemically with β-cyclodextrin

Electronic absorption spectra of charge-transfer complexes and effects of substituents in radical cations

Photochemical synthesis of cadmium sulfide nanoparticles

Photochemistry of trimethylene oxide and trimethylene sulfide radical cations in freonic matrices at 77 K

Properties of chemically generated π-radical cations and molecules of (meso-phenyl-β-octaethylporphyrinato)rhenium(V) with axial molecular oxygen

Synthesis and Properties of β-Oxo Sulfides of the Dioxothiolane Series

Environmentally benign synthesis of β-hydroxy sulfides using cyclic carbonates catalyzed by large-pore zeolites

Intermolecular complexes between sulfide radical cations from β-hydroxy sulfides and phosphate

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