NDLI: Catalytic Conversion of Simulated Biogas Mixtures to Synthesis Gas in a Fluidized Bed Reactor Supported by a DBD

Content Provider	Springer Nature Link
Author	Kroker, Thorsten Kolb, Torsten Schenk, Andreas Krawczyk, Krzysztof Młotek, Michal Gericke, Karl Heinz
Copyright Year	2012
Abstract	The catalytic conversion of methane and carbon dioxide was studied in a fluidized bed reactor supported by a 13.56 Hz driven coaxial DBD-reactor. Palladium or cupper catalyst which are covered on Al$_{2}$O$_{3}$ particles were used. The goal was to test whether biogas can be used for the production of synthesis gas. The influences of discharge power, catalysts and temperature of the catalyst bed on the product yield were studied. The starting material and product stream was analyzed by quadrupole mass spectrometry and infrared spectroscopy. H$_{2}$/CO ratios can be adjusted in a range between 0.65 (without a catalyst) and 1.75 (using a copper catalyst). The process is highly selective for hydrogen production (up to 83%, using a Palladium catalyst). A copper catalyst increases the H$_{2}$/CO ratio can from 1.04 to 1.16 and the palladium catalyst from 1.11 to 1.43 by heating the catalyst to a temperature of 250°C.
Starting Page	565
Ending Page	582
Page Count	18
File Format	PDF
ISSN	02724324
Journal	Plasma Chemistry and Plasma Processing
Volume Number	32
Issue Number	3
e-ISSN	15728986
Language	English
Publisher	Springer US
Publisher Date	2012-03-07
Publisher Place	Boston
Access Restriction	One Nation One Subscription (ONOS)
Subject Keyword	Biogas Cold plasma Fluidized bed reactor Synthesis gas Online monitoring Inorganic Chemistry Characterization and Evaluation of Materials Mechanics Nuclear Physics, Heavy Ions, Hadrons Mechanical Engineering
Content Type	Text
Resource Type	Article
Subject	Chemistry Surfaces, Coatings and Films Condensed Matter Physics Chemical Engineering

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4	Project PI / Joint PI	Principal Investigator and Joint Principal Investigators of the project	Dr. B. Sutradhar bsutra@ndl.gov.in Prof. Saswat Chakrabarti will be added soon
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