NDLI: Dry Reforming of Methane with Carbon Dioxide Using Pulsed DC Arc Plasma at Atmospheric Pressure

Content Provider	Springer Nature Link
Author	Yan, B. H. Wang, Q. Jin, Y. Cheng, Y.
Copyright Year	2010
Abstract	Dry reforming of CH$_{4}$ with CO$_{2}$ to produce syngas was investigated in a plasma reactor without catalysts at atmospheric pressure. The reactants passed through the plasma zone and reacted in milliseconds with high conversions and selectivity due to the localized high temperature. The results showed that both conversions and selectivity were higher when using a DC arc discharge than using a pulsed DC arc. Increasing the input energy density promoted the conversions of reactants. At an input power of 204 W, the conversions of CO$_{2}$ and CH$_{4}$ reached 99.3 and 99.6%, respectively, and the selectivity to products was almost 100%, where the molar ratio of CO$_{2}$/CH$_{4}$ was 1 with the reactants flow rate of 100 ml/min. Very little coke was formed during the course of reaction. Key parameters such as the pulse frequency, the input power and the total feed flow rate were studied to find the optimum operating condition.
Starting Page	257
Ending Page	266
Page Count	10
File Format	PDF
ISSN	02724324
Journal	Plasma Chemistry and Plasma Processing
Volume Number	30
Issue Number	2
e-ISSN	15728986
Language	English
Publisher	Springer US
Publisher Date	2010-02-06
Publisher Place	Boston
Access Restriction	One Nation One Subscription (ONOS)
Subject Keyword	Dry reforming Methane Carbon dioxide Pulsed DC arc plasma Syngas Nuclear Physics, Heavy Ions, Hadrons Inorganic Chemistry Mechanical Engineering Characterization and Evaluation of Materials Mechanics
Content Type	Text
Resource Type	Article
Subject	Chemistry Surfaces, Coatings and Films Condensed Matter Physics Chemical Engineering

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