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Catalytic activity of rare earth oxides in flameless methane combustion

Content Provider	Springer Nature Link
Author	Vishnyakov, A. V. Korshuva, I. A. Kochurikhin, V. E. Sal’nikova, L. S.
Copyright Year	2010
Abstract	The following rare earth oxides, which were prepared by the precipitation of hydroxides, were studied as catalysts for the reaction of complete methane oxidation: CeO$_{2}$, a hydrated phase of La$_{2}$O$_{3}$, Pr$_{6}$O$_{11}$, Tb$_{4}$O$_{7}$, and Gd$_{2}$O$_{3}$. The catalytic activities of the oxides were compared in terms of first-order reaction rate constants per unit surface area of the catalyst. With consideration for data on the reduction of CeO$_{2}$, Pr$_{6}$O$_{11}$, and Tb$_{4}$O$_{7}$, the previously proposed redox reaction mechanism on transition metal oxides was supported. The high activity of hydrated La$_{2}$O$_{3}$ was found, and it was hypothesized that, in this case, the process occurred by the mechanism of oxidative methane condensation followed by the rapid oxidation of the resulting intermediate products.
Starting Page	273
Ending Page	278
Page Count	6
File Format	PDF
ISSN	00231584
Journal	Kinetics and Catalysis
Volume Number	51
Issue Number	2
e-ISSN	16083210
Language	English
Publisher	SP MAIK Nauka/Interperiodica
Publisher Date	2010-04-24
Publisher Place	Dordrecht
Access Restriction	One Nation One Subscription (ONOS)
Subject Keyword	Physical Chemistry Catalysis
Content Type	Text
Resource Type	Article
Subject	Chemistry Catalysis Modeling and Simulation Computer Science Applications

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