NDLI: Nickel catalysts based on porous nickel for methane steam reforming

Content Provider	Springer Nature Link
Author	Sabirova, Z. A. Danilova, M. M. Zaikovskii, V. I. Kuzin, N. A. Kirillov, V. A. Kriger, T. A. Meshcheryakov, V. D. Rudina, N. A. Brizitskii, O. F. Khrobostov, L. N.
Copyright Year	2008
Abstract	The influence of synthesis conditions on the phase composition and texture of porous nickel supports as plates with a magnesium oxide underlayer were investigated by X-ray diffraction, low-temperature nitrogen absorption, and electron microscopy combined with X-ray microanalysis. Nickel catalysts supported on these plates were studied. Thermal treatment of Mg(NO$_{3}$)$_{2}$ in nitrogen yields a magnesium oxide underlayer with a small specific surface area (support I). The replacement of nitrogen with hydrogen leads to a larger surface area (support II). The formation of MgO is accompanied by the incorporation of Ni$^{2+}$ cations from the oxide film into the underlayer. Upon subsequent reduction with hydrogen or under the action of the reaction medium, these cations form fine crystallites of nickel. The supports having an oxide underlayer show a higher activity in methane steam reforming than the initial metallic nickel. Nickel catalysts on supports I and II show similar activities. The activity of the catalysts was stable throughout 50-h-long tests; no carbon deposits were detected by TEM.
Starting Page	428
Ending Page	434
Page Count	7
File Format	PDF
ISSN	00231584
Journal	Kinetics and Catalysis
Volume Number	49
Issue Number	3
e-ISSN	16083210
Language	English
Publisher	SP MAIK Nauka/Interperiodica
Publisher Date	2008-06-14
Publisher Place	Dordrecht
Access Restriction	One Nation One Subscription (ONOS)
Subject Keyword	Physical Chemistry Catalysis
Content Type	Text
Resource Type	Article
Subject	Chemistry Catalysis Modeling and Simulation Computer Science Applications

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