NDLI: Investigation of radionuclide $^{63}$Ni(II) sorption on ZSM-5 zeolite

Content Provider	Springer Nature Link
Author	Zhang, Hui Yu, Xianjin Chen, Lei Geng, Jiaqiang
Copyright Year	2010
Abstract	The sorption of $^{63}$Ni(II) from aqueous solution using ZSM-5 zeolite was investigated by batch technique under ambient conditions. ZSM-5 zeolite was characterized by point of zero net proton charge (PZNPC) titration. The sorption was investigated as a function of shaking time, pH, ionic strength, foreign ions, humic acid (HA), fulvic acid (FA) and temperature. The results indicate that the sorption of $^{63}$Ni(II) on ZSM-5 zeolite is strongly dependent on pH. The sorption is dependent on ionic strength at low pH, but independent of ionic strength at high pH values. The presence of HA/FA enhances $^{63}$Ni(II) sorption at low pH values, whereas reduces $^{63}$Ni(II) sorption at high pH values. The sorption isotherms are simulated by Langmuir model very well. The thermodynamic parameters (i.e., ∆H $^{0}$, ∆S $^{0}$ and ∆G $^{0}$) for the sorption of $^{63}$Ni(II) are determined from the temperature dependent sorption isotherms at 293.15, 313.15 and 333.15 K, respectively, and the results indicate that the sorption process of $^{63}$Ni(II) on ZSM-5 zeolite is spontaneous and endothermic.
Starting Page	249
Ending Page	258
Page Count	10
File Format	PDF
ISSN	02365731
Journal	Journal of Radioanalytical and Nuclear Chemistry
Volume Number	286
Issue Number	1
e-ISSN	15882780
Language	English
Publisher	Springer Netherlands
Publisher Date	2010-06-22
Publisher Place	Dordrecht
Access Restriction	One Nation One Subscription (ONOS)
Subject Keyword	$^{63}$Ni(II) ZSM-5 zeolite Sorption pH Thermodynamic parameter Inorganic Chemistry Diagnostic Radiology Nuclear Physics, Heavy Ions, Hadrons Physical Chemistry Nuclear Chemistry
Content Type	Text
Resource Type	Article
Subject	Spectroscopy Pollution Health, Toxicology and Mutagenesis Radiology, Nuclear Medicine and Imaging Analytical Chemistry Public Health, Environmental and Occupational Health Nuclear Energy and Engineering

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