NDLI: Nitroxyls and PELDOR: Nitroxyl radicals in pulsed electron-electron double resonance spectroscopy

Content Provider	Springer Nature Link
Author	Tsvetkov, Yu. D.
Copyright Year	2013
Abstract	The review considers the main propositions of PELDOR theory. It is shown how from the analysis of PELDOR time traces it is possible to find the parameters of a spin system such as the distance and the distance distribution (spectrum), number of spins in aggregates and complexes, exchange integral and how to separate for the following analysis the inter- and intramolecular contributions to the general dipole interaction. Examples of PELDOR application in the studies of the spatial distribution of nitroxyl radicals, the charge effect of dipolar interacting nitroxyls on their spatial distribution are given and the results of the determination of distances and the spectrum of distances for nitroxyl bi-, tri-, and tetraradicals are presented. The works on nitroxyl radicals in which the orientation selectivity effect, spin exchange, and conformational properties of the radicals are examined by the PELDOR method are analyzed. The studies of the structure of paramagnetic ion-nitroxyl radical pairs and the PELDOR data on nitroxyls at high frequencies (high fields) are considered. The last section of the review is devoted to the works examining the properties such as the molecular flexibility of oligomers and supramolecules contains nitroxyl radicals.
Starting Page	42
Ending Page	72
Page Count	31
File Format	PDF
ISSN	00224766
Journal	Journal of Structural Chemistry
Volume Number	54
Issue Number	1
e-ISSN	15738779
Language	English
Publisher	Springer US
Publisher Date	2013-10-11
Publisher Place	Boston
Access Restriction	One Nation One Subscription (ONOS)
Subject Keyword	EPR PELDOR nitroxyls dipole magnetic interactions distances spectrum of distances Inorganic Chemistry Physical Chemistry Atomic, Molecular, Optical and Plasma Physics Atomic/Molecular Structure and Spectra Solid State Physics
Content Type	Text
Resource Type	Article
Subject	Materials Chemistry Physical and Theoretical Chemistry Inorganic Chemistry

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