NDLI: Crisis of stability of hydration shell of Na+ ion in condensing water vapor

Content Provider	Springer Nature Link
Author	Shevkuv, S. V.
Copyright Year	2011
Abstract	The Gibbs energy and equilibrium work of the formation of nuclei of the condensed phase on sodium ions are calculated on the molecular level by a Monte Carlo simulation using a detailed interaction model. The stationary rate of nucleation is estimated based on the data obtained. The presence of ionic impurities only substantially affects the rate of nucleation at strong vapor supersaturation. The nucleus losses its thermodynamic stability with an increase in the size of the nucleus and the barrier is formed depending on the work of formation on the size of the nucleus. An abrupt loss of stability is accompanied by pushing the ion off of the microdroplet surface and the restoration of the network of hydrogen bonds. The effect of pushing an ion to the surface of a cluster greatly depends on many-particle polarization interactions.
Starting Page	275
Ending Page	286
Page Count	12
File Format	PDF
ISSN	1061933X
Journal	Colloid Journal
Volume Number	73
Issue Number	2
e-ISSN	16083067
Language	English
Publisher	SP MAIK Nauka/Interperiodica
Publisher Date	2011-04-16
Publisher Place	Dordrecht
Access Restriction	One Nation One Subscription (ONOS)
Subject Keyword	Polymer Sciences Surfaces and Interfaces, Thin Films
Content Type	Text
Resource Type	Article
Subject	Colloid and Surface Chemistry Physical and Theoretical Chemistry Surfaces and Interfaces

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Crisis of stability of hydration shell of Na+ ion in condensing water vapor