NDLI: Effect of support on the conversion of methane to synthesis gas over supported iridium catalysts

Content Provider	Springer Nature Link
Author	Nakagawa, Kiyoharu Anzai, Kengo Matsui, Naoko Ikenaga, Naoki Suzuki, Toshimitsu Teng, Yonghong Kobayashi, Tetsuhiko Haruta, Masatake
Copyright Year	1998
Abstract	A partial oxidation of methane was carried out using iridium catalysts supported on several metal oxides. The productivity of the synthesis gas from methane was strongly affected by the choice of support oxides for the catalysts. The synthesis gas production proceeded basically via a two-step reaction consisting of methane combustion to give H2O and CO2, followed by the reforming of methane from CO2 and steam. Although the combustion and the reforming of methane from steam did not depend upon the catalyst support, a large variation in the catalytic activity for the reforming of methane from CO2 was observed over Ir catalysts with different supports. The support activity order in the reforming of methane from CO2 with iridium catalysts was as follows: TiO2≧ZrO2≧Y2O3>La2O3>MgO≧Al2O3>SiO2. The same order was observed in the synthesis gas production from the partial oxidation of methane.
Starting Page	163
Ending Page	167
Page Count	5
File Format	PDF
ISSN	1011372X
Journal	Catalysis Letters
Volume Number	51
Issue Number	3-4
e-ISSN	1572879X
Language	English
Publisher	Kluwer Academic Publishers-Plenum Publishers
Publisher Date	1998-01-01
Publisher Place	New York
Access Restriction	One Nation One Subscription (ONOS)
Subject Keyword	Physical Chemistry Industrial Chemistry/Chemical Engineering Catalysis Pharmacy
Content Type	Text
Resource Type	Article
Subject	Chemistry Catalysis

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