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| Content Provider | Springer Nature Link |
|---|---|
| Author | Deroche, Irena Gaberova, Lucia Maurin, Guillaume Llewellyn, Philip Castro, Maria Wright, Paul |
| Copyright Year | 2008 |
| Abstract | The adsorption properties of carbon dioxide in SAPO STA-7 has been investigated by combining Grand Canonical Monte Carlo simulation and microcalorimetry. The modeling approach, based on both newly derived interatomic potentials for describing the interaction between CO2 and the Brønsted acid sites, and a realistic description of the silicon distribution within the framework, provides isotherms and evolutions of the differential enthalpy of adsorption as a function of coverage for the STA-7 material characterised by a silicon fraction of 0.19. The simulated results are revealed to be in good agreement with the experimental data that allowed us to provide a possible microscopic mechanism of CO2 adsorption in this material. These whole results are thus compared to those obtained for the purely aluminophosphate form of the AlPO-18. It is clearly emphasized that distinct adsorption behaviours are observed in these two systems, depending on the energetic characteristics of their surfaces. |
| Starting Page | 207 |
| Ending Page | 213 |
| Page Count | 7 |
| File Format | |
| ISSN | 09295607 |
| Journal | Adsorption |
| Volume Number | 14 |
| Issue Number | 2-3 |
| e-ISSN | 15728757 |
| Language | English |
| Publisher | Springer US |
| Publisher Date | 2008-01-09 |
| Publisher Place | Boston |
| Access Restriction | One Nation One Subscription (ONOS) |
| Subject Keyword | SAPO STA-7 AlPO-18 CO2 Adsorption Grand Canonical Monte Carlo Microcalorimetry Isotherms and enthalpies of adsorption Engineering Thermodynamics, Transport Phenomena Industrial Chemistry/Chemical Engineering Surfaces and Interfaces, Thin Films |
| Content Type | Text |
| Resource Type | Article |
| Subject | Chemistry Chemical Engineering Surfaces and Interfaces |
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