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Enhanced photovoltaic performance of quasi-solid-state dye-sensitized solar cells via incorporating quaternized ammonium iodide-containing conjugated polymer into PEO gel electrolytes

Content Provider	Springer Nature Link
Author	Lee, Rong Ho Cheng, Tun Fang Chang, Jhih Wei Ho, Jhu Heng
Copyright Year	2011
Abstract	In this study, a series of gel electrolytes prepared from blends of alternating conjugated polymer electrolytes (CPEs)/poly(ethylene oxide) (PEO) were developed for use in quasi-solid-state dye-sensitized solar cells (DSSCs). The alternating CPEs poly[(N-(3′-((N,N-dimethyl)-N-ethylammonium)propyl)-3,6-carbazole)-alt-(9,9-dioctyl-2,7-fluorene)]diiodide, poly[(N-(3′-((N,N-dimethyl)-N-ethylammonium)propyl)-3,6-carbazole)-alt-(9,9-bis(2-(2-methoxyethoxy)ethyl)-2,7-fluorene)]diiodide (MPCFO-E), and poly[(N-(3′-((N,N-dimethyl)-N-ethylammonium)propyl)-3,6-carbazole)-alt-(siloxane substituted-2,7-fluorene)]diiodide (MPCFS-E) were synthesized through copolymerization of carbazole units (featuring quaternized ammonium iodide groups) and fluorene units featuring flexible side chains (9,9-dioctylfluorene, ethylene oxide-substituted fluorene, and siloxane-substituted fluorene, respectively). The MPCFO-E/PEO-based and MPCFS-E/PEO-based DSSCs exhibited lower electrochemical resistances, superior photovoltaic (PV) properties, and improved PV stabilities relative to those of the corresponding PEO-based DSSC. Among the studied systems, the DSSC based on the MPCFO-E (0.5 wt.%)/PEO blend electrolyte exhibited the best PV performance, with a short current density of 4.97 mA cm−2 and a photoenergy conversion efficiency of 1.17%.
Starting Page	817
Ending Page	829
Page Count	13
File Format	PDF
ISSN	0303402X
Journal	Colloid and Polymer Science
Volume Number	289
Issue Number	7
e-ISSN	14351536
Language	English
Publisher	Springer-Verlag
Publisher Date	2011-03-04
Publisher Place	Berlin/Heidelberg
Access Restriction	One Nation One Subscription (ONOS)
Subject Keyword	Dye-sensitized solar cell Conjugated polymer electrolyte Polymer gel electrolyte Photovoltaic property Photoconversion efficiency Polymer Sciences Physical Chemistry Soft and Granular Matter, Complex Fluids and Microfluidics Food Science Characterization and Evaluation of Materials
Content Type	Text
Resource Type	Article
Subject	Colloid and Surface Chemistry Materials Chemistry Physical and Theoretical Chemistry Polymers and Plastics

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