NDLI: Correlation between photoluminescence, optical and structural properties of amorphous nitrogen-rich carbon nitride films

Content Provider	Springer Nature Link
Author	Plass, M.F. Popov, C. Ivav, B. Mändl, S. Jelinek, M. Zambov, L.M. Kulisch, W.
Copyright Year	2000
Abstract	Amorphous nitrogen-rich carbon nitride (CNx) films have been prepared by inductively coupled plasma chemical vapour deposition (ICP-CVD) utilizing transport reactions from a solid carbon source. The nitrogen atomic fraction N/(C+N) is about 1 or even higher as detected by various surface and bulk sensitive methods. An investigation of the chemical bonding structure showed that the films are composed of >C=N units with a small fraction of C≡N groups. Based on these findings, several structural units derived from cis- and trans-conjugated carbon–nitrogen chains are proposed. The optical properties of the CNx films were studied by transmission spectroscopy and spectral ellipsometry; the optical Tauc gap was determined to 2.1±0.05 eV. The photoluminescence characteristics were measured at three different excitation wavelengths (476, 488 and 515 nm) and revealed two individual contributions. These data are interpreted in terms of the different structural units comprising the nitrogen-rich CNx films.
Starting Page	21
Ending Page	27
Page Count	7
File Format	PDF
ISSN	09478396
Journal	Applied Physics A
Volume Number	72
Issue Number	1
e-ISSN	14320630
Language	English
Publisher	Springer-Verlag
Publisher Date	2001-01-01
Publisher Place	Berlin, Heidelberg
Access Restriction	One Nation One Subscription (ONOS)
Content Type	Text
Resource Type	Article
Subject	Chemistry Materials Science

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