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| Content Provider | Springer Nature Link |
|---|---|
| Author | Chen, Bingyu Liu, Guijian Sun, Ruoyu |
| Copyright Year | 2016 |
| Abstract | A better understanding on the partitioning behavior of mercury (Hg) during coal combustion in large-scale coal-fired power plants is fundamental for drafting Hg-emission control regulations. Two large coal-fired utility boilers, equipped with electrostatic precipitators (ESPs) and a wet flue gas desulfurization (WFGD) system, respectively, in coal energy-dominant Huainan City, China, were selected to investigate the distribution and fate of Hg during coal combustion. In three sampling campaigns, we found that Hg in bottom ash was severely depleted with a relative enrichment (RE) index <7 %, whereas the RE index for fly ash (9–54 %) was comparatively higher and variable. Extremely high Hg was concentrated in gypsum (≤4500 ng/g), which is produced in the WFGD system. Mass balance calculation shows that the shares of Hg in bottom ash, fly ash, WFGD products (gypsum, effluents, sludge), and stack emissions were <2, 17–32, 7–22, and 54–82 %, respectively. The Hg-removal efficiencies of ESPs, WFGD, and ESPs + WFGD were 17–32, 10–29, and 36–46 %, respectively. The Hg-emission factor of studied boilers was in a high range of 0.24–0.29 g Hg/t coal. We estimated that Hg emissions in all Huainan coal-fired power plants varied from 1.8 Mg in 2003 to 7.3 Mg in 2010. |
| Starting Page | 724 |
| Ending Page | 733 |
| Page Count | 10 |
| File Format | |
| ISSN | 00904341 |
| Journal | Archives of Environmental Contamination and Toxicology |
| Volume Number | 70 |
| Issue Number | 4 |
| e-ISSN | 14320703 |
| Language | English |
| Publisher | Springer US |
| Publisher Date | 2016-02-16 |
| Publisher Place | New York |
| Access Restriction | One Nation One Subscription (ONOS) |
| Subject Keyword | Ecotoxicology Pollution Environmental Health Environmental Chemistry Soil Science & Conservation Environmental Monitoring/Analysis |
| Content Type | Text |
| Resource Type | Article |
| Subject | Pollution Health, Toxicology and Mutagenesis Medicine Toxicology |
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