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Ship-based MAX-DOAS measurements of tropospheric NO2 and SO2 in the South China and Sulu Sea
| Content Provider | Semantic Scholar |
|---|---|
| Author | Schreier, Stefan F. Peters, E. M. Richter, Andreas M. Lampel, Johannes Wittrock, Folkard Burrows, John P. |
| Copyright Year | 2015 |
| Abstract | In November 2011, ship-based Multi-Axis Differential Optical Absorption Spectroscopy (MAX-DOAS) measurements were performed within the SHIVA campaign on board RV Sonne in the South China and Sulu Sea. Spectral measurements for a total of eleven days could be used to retrieve tropospheric slant column densities (SCDs) of nitrogen dioxide (NO2) and sulfur dioxide (SO2) in the marine environment. The NO2 fit was performed following recommendations developed during the CINDI campaign and adapted for the ship-based measurements. We found that the inclusion of a cross section for liquid water and an empirical correction spectrum accounting for the effects of liquid water and vibrational Raman scattering (VRS) slightly improved the NO2 fit quality, especially at lower elevation angles and for lower NO2 levels. The conversion of SCDs into tropospheric NO2 vertical columns (TVC NO2) has been achieved using both a simple geometric approach and the Bremian advanced MAX-DOAS Retrieval Algorithm (BREAM), which is based on the optimal estimation method and accounts for atmospheric radiative transfer. We found good agreement between the geometric approach using the 15 |
| Starting Page | 331 |
| Ending Page | 343 |
| Page Count | 13 |
| File Format | PDF HTM / HTML |
| DOI | 10.1016/j.atmosenv.2014.12.015 |
| Volume Number | 102 |
| Alternate Webpage(s) | http://www.doas-bremen.de/paper/ae_15_schreier.pdf |
| Alternate Webpage(s) | https://doi.org/10.1016/j.atmosenv.2014.12.015 |
| Language | English |
| Access Restriction | Open |
| Content Type | Text |
| Resource Type | Article |