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Nonclassical photon statistics in single-molecule fluorescence at room temperature
| Content Provider | Semantic Scholar |
|---|---|
| Author | Fleury Segura Zumofen Hecht, Stefan Wild |
| Copyright Year | 2000 |
| Abstract | The fluorescence of single terrylene molecules in a crystalline host is investigated at room temperature by scanning confocal optical microscopy. Photon arrival times are analyzed in terms of interphoton time distributions, second order correlation functions, and the variance of the photon number probability distribution. Antibunching at short times and bunching behavior for longer times is observed, associated with sub- and super-Poissonian statistics, respectively. A rate-equation analysis of the molecular level populations indicates an accelerated reverse intersystem crossing. |
| File Format | PDF HTM / HTML |
| DOI | 10.1016/S0022-2313(01)00367-2 |
| PubMed reference number | 11017465 |
| Journal | Medline |
| Volume Number | 84 |
| Issue Number | 6 |
| Alternate Webpage(s) | https://www.photonics.ethz.ch/fileadmin/user_upload/Courses/NanoOptics/ProjectReports/hecht00.pdf |
| Alternate Webpage(s) | https://doi.org/10.1016/S0022-2313%2801%2900367-2 |
| Journal | Physical review letters |
| Language | English |
| Access Restriction | Open |
| Content Type | Text |
| Resource Type | Article |