NDLI: Methane oxidation over Pt/Al 2 O 3 and Pd/Al 2 O 3 catalysts u

Content Provider	Semantic Scholar
Author	Carlsson, Per-Anders Fridell, Erik Skoglundh, Magnus
Copyright Year	2007
Abstract	We communicate experimental results for the oxidation of methane by oxygen over alumina supported Pd and Pt monolith catalysts under transient conditions. Temperature programmed reaction (TPReaction) and reactant pulse-response (PR) experiments have been performed, using a continuous gas-flow reactor equipped with a downstream mass spectrometer for gas phase analysis. Special attention was paid to the influence of gas composition changes, i.e. O2 and H2 pulsing, respectively, on the methane conversion. For Pt/Al2O3 oxygen pulsing can significantly increase the methane conversion which can be even further improved by pulsing hydrogen instead. Such transient effects are not observed for the Pd/Al2O3 catalyst for which instead constantly lean conditions is beneficial. Our results suggest that under lean conditions
File Format	PDF HTM / HTML
Alternate Webpage(s)	https://research.chalmers.se/publication/26180/file/26180_Fulltext.pdf
Language	English
Access Restriction	Open
Content Type	Text
Resource Type	Article

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