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Rapid formation of black titania photoanodes: pulsed laser-induced oxygen release and enhanced solar water splitting efficiency
| Content Provider | Semantic Scholar |
|---|---|
| Author | Nakajima, Tomohiko Nakamura, Tomoaki Shinoda, Kentaro Tsuchiya, Tetsuo |
| Copyright Year | 2014 |
| Abstract | Solar energy is a key part of creating a sustainable society. Pulsed ultraviolet laser irradiation of titania films is a simple process for making oxygen-deficient black titania (TiO2−x) films that use the solar spectrum efficiently. TiO2−x photoanodes were obtained by KrF laser irradiation under low-vacuum conditions for several minutes. The TiO2−x film had a larger absorbance than pristine TiO2 in the visible light region, and it exhibited a substantial increase in photoelectrochemical water splitting under simulated solar light. The solar-to-hydrogen efficiency of the TiO2−x photoanode reached 0.52%, which was 2.6-fold higher than that of the pristine TiO2 photoanode. This rapid fabrication process for black titania photoanodes has great potential for industrial solar hydrogen production. |
| Starting Page | 6762 |
| Ending Page | 6771 |
| Page Count | 10 |
| File Format | PDF HTM / HTML |
| DOI | 10.1039/C4TA00557K |
| Alternate Webpage(s) | https://pubs.rsc.org/en/content/getauthorversionpdf/C4TA00557K |
| Alternate Webpage(s) | http://www.rsc.org/suppdata/ta/c4/c4ta00557k/c4ta00557k1.pdf |
| Alternate Webpage(s) | https://doi.org/10.1039/C4TA00557K |
| Volume Number | 2 |
| Language | English |
| Access Restriction | Open |
| Content Type | Text |
| Resource Type | Article |