NDLI: Effects of Energy Exchange on Vibrational Dephasing Times in Raman Scattering

Content Provider	Semantic Scholar
Author	Harris, Charles Bonner Shelby, Robert M. Cornelius, Paul A.
Copyright Year	1977
Abstract	It is shown that the Raman lineshape function and/or vibrational dephasing times can reflect random frequency modulation of high frequency vibrational modes via exchange with low frequency modes. When exchange is i_ncorporated into the vibrational correlation function, lifetimes and scattering rates between modes can be quantitatively determined from the temperature dependence of the spontaneous Raman spectrum. Finally, some experimental results on vibrational redistribution are presented which demonstrate the salient features of the theory.
Starting Page	1415
Ending Page	1419
Page Count	5
File Format	PDF HTM / HTML
DOI	10.1103/PhysRevLett.38.1415
Alternate Webpage(s)	https://cloudfront.escholarship.org/dist/prd/content/qt2c49m1qz/qt2c49m1qz.pdf?t=p2bfvj
Alternate Webpage(s)	https://doi.org/10.1103/PhysRevLett.38.1415
Volume Number	38
Language	English
Access Restriction	Open
Content Type	Text
Resource Type	Article

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