NDLI: Tandem Ring-Opening-Ring-Closing Metathesis for Functional Metathesis Catalysts.

Content Provider	Semantic Scholar
Author	Nagarkar, Amit A. Yasir, Mohammad Crochet, Aurelien Fromm, Katharina M. Kilbinger, Andreas F. M.
Copyright Year	2016
Abstract	Use of a tandem ring-opening-ring-closing metathesis (RORCM) strategy for the synthesis of functional metathesis catalysts is reported. Ring opening of 7-substituted norbornenes and subsequent ring-closing metathesis forming a thermodynamically stable 6-membered ring lead to a very efficient synthesis of new catalysts from commercially available Grubbs' catalysts. Hydroxy functionalized Grubbs' first- as well as third-generation catalysts have been synthesized. Mechanistic studies have been performed to elucidate the order of attack of the olefinic bonds. This strategy was also used to synthesize the ruthenium methylidene complex.
File Format	PDF HTM / HTML
DOI	10.1002/anie.201604112
PubMed reference number	27592840
Journal	Medline
Volume Number	55
Issue Number	40
Alternate Webpage(s)	http://doc.rero.ch/record/278539/files/kil_tro_sm.pdf
Alternate Webpage(s)	http://doc.rero.ch/record/278539/files/kil_tro.pdf
Alternate Webpage(s)	https://doi.org/10.1002/anie.201604112
Journal	Angewandte Chemie
Language	English
Access Restriction	Open
Content Type	Text
Resource Type	Article

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