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Magnetic ordering and charge dynamics in κ-(BEDT-TTF)2Cu[N(CN)2]Cl.
| Content Provider | Semantic Scholar |
|---|---|
| Author | Tomi'c, S. Pinterić, Marko Ivek, Tomislav Sedlmeier, K. Beyer, R. Wu, Da-Zhi Schlueter, John A. Schweitzer, D. Dressel, Martin |
| Copyright Year | 2013 |
| Abstract | The Mott insulator κ-(BEDT-TTF)2Cu[N(CN)2]Cl consists of molecular dimers arranged on an anisotropic triangular lattice. At low temperatures a pronounced dielectric anomaly is observed, and eventually a canted antiferromagnetic ground state forms. Optical spectroscopy clearly rules out charge imbalance and the existence of quantum electric dipoles with a dipolar-spin coupling. Here we suggest a novel form of spin-charge coupling where the prominent in-plane dielectric response in κ-(BEDT-TTF)2Cu[N(CN)2]Cl is explained by short-range discommensurations of the antiferromagnetic phase in the temperature range 30 K < T < 50 K, and by relaxation of charged domain walls in the ferromagnetic structure at lower temperatures. |
| Starting Page | 436004 |
| Ending Page | 436004 |
| Page Count | 1 |
| File Format | PDF HTM / HTML |
| DOI | 10.1088/0953-8984/25/43/436004 |
| PubMed reference number | 24107640 |
| Journal | Medline |
| Volume Number | 25 |
| Issue Number | 43 |
| Alternate Webpage(s) | http://bib.irb.hr/datoteka/647308.STETCl_JPCM2013.pdf |
| Alternate Webpage(s) | https://doi.org/10.1088/0953-8984%2F25%2F43%2F436004 |
| Journal | Journal of physics. Condensed matter : an Institute of Physics journal |
| Language | English |
| Access Restriction | Open |
| Content Type | Text |
| Resource Type | Article |