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Enhancing performance and uniformity of CH3NH3PbI3−xClx perovskite solar cells by air-heated-oven assisted annealing under various humidities
| Content Provider | Semantic Scholar |
|---|---|
| Author | Zhou, Qing Jin, Zhiwen Wang, Jizheng |
| Copyright Year | 2016 |
| Abstract | UNLABELLED To fabricate high-performance metal-halide perovskite solar cells, a thermal annealing process is indispensable in preparing high quality perovskite film. And usually such annealing is performed on hot plate. However hot-plate annealing could cause problems such as inhomogeneous heating (induced by non-tight contact between the sample and the plate), it is also not fit for large scale manufactory. In this paper, we conduct the annealing process in air-heated oven under various humidity environments, and compared the resulted films (CH3NH3PbI(3-x)Cl(x)) and devices (Al/PC61BM/CH3NH3PbI(3-x)Cl(x)/ PEDOT PSS/ITO/glass) with that obtained via hot-plate annealing. It is found that the air-heated-oven annealing is superior to the hot-plate annealing: the annealing time is shorter, the films are more uniform, and the devices exhibit higher power conversion efficiency and better uniformity. The highest efficiencies achieved for the oven and hot-plate annealing processes are 14.9% and 13.5%, and the corresponding standard deviations are 0.5% and 0.8%, respectively. Our work here indicates that air-heated-oven annealing could be a more reliable and more efficient way for both lab research and large-scale production. |
| File Format | PDF HTM / HTML |
| DOI | 10.1038/srep21257 |
| PubMed reference number | 26879260 |
| Journal | Medline |
| Volume Number | 6 |
| Alternate Webpage(s) | https://media.nature.com/original/nature-assets/srep/2016/160216/srep21257/extref/srep21257-s1.pdf |
| Alternate Webpage(s) | https://doi.org/10.1038/srep21257 |
| Journal | Scientific reports |
| Language | English |
| Access Restriction | Open |
| Content Type | Text |
| Resource Type | Article |