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n nanotube aerogel – Pt nanocomposites toward enhanced energy conversion in dye-sensitized solar cells
| Content Provider | Semantic Scholar |
|---|---|
| Author | Chen, Haijun Ren, Jing He, Hongcai Cao, Yonghai Wang, Ning Guo, Zhanhu |
| Copyright Year | 2016 |
| Abstract | With the lab-made carbon nanotube aerogel (CNA) serving as the counter electrode (CE), dye-sensitized solar cells (DSSCs) operated under solar simulator illumination (100 mW cm , AM 1.5 G) demonstrated an overall power conversion efficiency (h) of 8.35%, higher than the h of 5.95 and 7.39% of DSSCs with a multi-walled carbon nanotube (MWCNT) CE and conventional Pt CE, respectively. With only 3.75 wt% Pt nanoparticles to form an aerogel carbon nanotube composite (CNA-3.75 wt% Pt) CE, the corresponding h was further increased to 9.04%. The enhanced performance by introducing Pt nanoparticles is mainly attributed to the improved electrocatalytic activity, reduced charge-transfer resistance (Rct) at the CE/electrolyte interface, and increased diffusion for the redox couple in the electrolyte. This work provides substantial support for developing lowcost Pt-loaded nanocomposite CEs to further enhance the DSSC performance. |
| File Format | PDF HTM / HTML |
| Alternate Webpage(s) | http://composites.utk.edu/papers%20in%20pdf/JMCA_CNTs_Pt.pdf |
| Language | English |
| Access Restriction | Open |
| Content Type | Text |
| Resource Type | Article |