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Phonon-induced population dynamics and intersystem crossing in nitrogen-vacancy centers.
| Content Provider | Semantic Scholar |
|---|---|
| Author | Sipahigil, Alp Doherty, Marcus William Markham, Matthew Kubanek, Alexander |
| Copyright Year | 2015 |
| Abstract | We report direct measurement of population dynamics in the excited state manifold of a nitrogen-vacancy (NV) center in diamond. We quantify the phonon-induced mixing rate and demonstrate that it can be completely suppressed at low temperatures. Further, we measure the intersystem crossing (ISC) rate for different excited states and develop a theoretical model that unifies the phonon-induced mixing and ISC mechanisms. We find that our model is in excellent agreement with experiment and that it can be used to predict unknown elements of the NV center's electronic structure. We discuss the model's implications for enhancing the NV center's performance as a room-temperature sensor. |
| Starting Page | 145502 |
| Ending Page | 145502 |
| Page Count | 1 |
| File Format | PDF HTM / HTML |
| Alternate Webpage(s) | http://ciqm.harvard.edu/uploads/2/3/3/4/23349210/goldman_arxiv_1406.4065.pdf |
| Alternate Webpage(s) | http://ciqm.harvard.edu/uploads/2/3/3/4/23349210/goldman2015.pdf |
| PubMed reference number | 25910136v1 |
| Volume Number | 114 |
| Issue Number | 14 |
| Journal | Physical review letters |
| Language | English |
| Access Restriction | Open |
| Subject Keyword | Blood urea nitrogen measurement Cold Temperature Cross Infection Diamond Phonons manifold |
| Content Type | Text |
| Resource Type | Article |