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$g-C_{3}N_{4}/Pt/BiVO_{4}$ nanocomposites for highly efficient visible-light photocatalytic removal of contaminants and hydrogen generation
| Content Provider | Scilit |
|---|---|
| Author | Si, Yun-Hui Chen, Wei-Min Shang, Shao-Ke Xia, Yu Zeng, Xie-Rong Zhou, Ji Li, Ya-Yun |
| Copyright Year | 2019 |
| Description | Journal: Nanotechnology Inspired by natural photosynthesis, the artificial heterojunction photocatalysts have been extensively studied. Herein, a novel ternary g-C3N4/Pt/BiVO4 photocatalytic system was successfully synthesized, where Pt@BiVO4 nanosheet is anchored on the surface of layered graphitic carbon nitride (g-C3N4) as evidenced by structural observations. Ultraviolet photoelectron spectroscopy (UPS) and UV-Visible diffuse reflectance spectroscopy (UV-vis DRS) are carried out to identify the position of the conduction band (CB) and valence band (VB). A Z-scheme is used to interpret the superior photocatalytic performance of g-C3N4/Pt/BiVO4 and further verified by the capture of free radicals and terephthalic acid photoluminescence experiments. Compared with the g-C3N4/BiVO4 binary system, the Z-scheme g-C3N4/Pt/BiVO4 photocatalyst possesses not only enhanced carriers separation efficiency but also maintains sufficient redox properties, thus inducing the superior photocatalytic activity. More importantly, the novel Z-scheme photocatalyst exhibit excellent recycle stability, which can provide inspiration on the rational design of efficient and practical photocatalyst in environmental pollution treatment. Ternary photocatalyst also exhibits significantly enhanced visible-light photocatalytic hydrogen production performance. |
| Related Links | https://iopscience.iop.org/article/10.1088/1361-6528/ab5bc5/pdf |
| ISSN | 09574484 |
| e-ISSN | 13616528 |
| DOI | 10.1088/1361-6528/ab5bc5 |
| Journal | Nanotechnology |
| Issue Number | 12 |
| Volume Number | 31 |
| Language | English |
| Publisher | IOP Publishing |
| Publisher Date | 2019-11-26 |
| Access Restriction | Open |
| Subject Keyword | Journal: Nanotechnology Chemical Engineering Environmental Sciences |
| Content Type | Text |
| Resource Type | Article |
| Subject | Chemistry Nanoscience and Nanotechnology Mechanics of Materials Mechanical Engineering Bioengineering Electrical and Electronic Engineering |