NDLI: Nitrogen-enriched hierarchically porous carbon materials fabricated by graphene aerogel templated Schiff-base chemistry for high performance electrochemical capacitors

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Polymer Chemistry Vol - 6 Issue - 6

Polymer Chemistry Vol - 6 Issue - 5

Polymer Chemistry Vol -5

Polymer Chemistry Vol -4

Polymer Chemistry Vol -3

Polymer Chemistry Vol -2

Polymer Chemistry Vol -1

Nitrogen-enriched hierarchically porous carbon materials fabricated by graphene aerogel templated Schiff-base chemistry for high performance electrochemical capacitors

Content Provider	Royal Society of Chemistry (RSC)
Author	Zhuang, Xiaodong Mai, Yiyong Huang, Yinjuan Feng, Xinliang Wu, Dongqing Yang, Xiangwen Jiang, Jianzhong Tian, Hao Zhang, Fan
Copyright Year	2015
Abstract	This article presents a facile and effective approach for synthesizing three-dimensional (3D) graphene-coupled Schiff-base hierarchically porous polymers (GS-HPPs). The method involves the polymerization of melamine and 1,4-phthalaldehyde, yielding Schiff-base porous polymers on the interconnected macroporous frameworks of 3D graphene aerogels. The as-synthesized GS-HPPs possess hierarchically porous structures containing macro-/meso-/micropores, along with large specific surface areas up to 776 m2 g−1 and high nitrogen contents up to 36.8 wt%. Consequently, 3D nitrogen-enriched hierarchically porous carbon (N-HPC) materials with macro-/meso-/micropores were obtained by the pyrolysis of the GS-HPPs at a high temperature of 800 °C under a nitrogen atmosphere. With a hierarchically porous structure, good thermal stability and a high nitrogen-doping content up to 7.2 wt%, the N-HPC samples show a high specific capacitance of 335 F g−1 at 0.1 A g−1 in 6 M KOH, a good capacitance retention with increasing current density, and an outstanding cycling stability. The superior electrochemical performance means that the N-HPC materials have great potential as electrode materials for supercapacitors.
Starting Page	1088
Ending Page	1095
Page Count	8
File Format	HTM / HTML PDF
ISSN	17599954
Volume Number	6
Issue Number	7
Journal	Polymer Chemistry
DOI	10.1039/c4py01408a
Language	English
Publisher	Royal Society of Chemistry
Access Restriction	Open
Subject Keyword	Pyrolysis Electrode Graphene Polymerization Electrochemistry Capacitance Melamine resin Nitrogen Carbon Current density Three-dimensional space
Content Type	Text
Resource Type	Article
Subject	Organic Chemistry Biochemistry Bioengineering Biomedical Engineering Polymers and Plastics

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