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Journal of Materials Chemistry C Vol - 3 Issue - 8

Journal of Materials Chemistry C Vol - 3 Issue - 7

Journal of Materials Chemistry C Vol - 3 Issue - 6

Journal of Materials Chemistry C Vol - 3 Issue - 5

Journal of Materials Chemistry C Vol -2

Journal of Materials Chemistry C Vol -1

Fluorescent probes for “off–on” sensitive and selective detection of mercury ions and l-cysteine based on graphitic carbon nitride nanosheets

Content Provider	Royal Society of Chemistry (RSC)
Author	Huang, Zhouyi Zhang, Hanqiang Zhang, Wuxiang Huang, Qitong Hao, Aiyou Kang, Lianping Huang, Yihong Hu, Shirong Wei, Chan
Copyright Year	2015
Abstract	A novel approach for preparation of graphitic carbon nitride nanosheets (CNNS) from stripping graphitic carbon nitride by strong acid and ultrasonic technology was demonstrated in this study for the first time. Transmission electron microscopy (TEM) was employed to characterize the surface morphology. Atomic force microscope (AFM) was carried out to characterize the thickness of nanosheets. X-Ray diffraction (XRD) was performed to estimate the lattice structure. X-Ray photoelectron spectroscopy (XPS) was carried out to characterize the surface composition and element analysis. Fourier transform infrared spectroscopy (FT-IR) was allowed to identify the functional groups. The as-synthesized CNNS exhibited excellent emission property as well as excitation-independent emission behavior, and fluorescence quantum yields could reach approximately 12.53%. Mercury ion (Hg2+) can make a result of quenching the significant intensity of fluorescence of CNNS by formation of a covalent bond between empty orbital of Hg2+ and the π electrons of N (turn-off). Moreover, the addition of the L-cysteine (L-Cys) can enhance the intensity of fluorescence of the CNNS– Hg2+ system through the thiol group of L-Cys anchored with Hg2+ and drag it from the surface of CNNS (turn-on). The CNNS was consequently functioned as a fluorescence probe towards “off–on” detection of Hg2+ and L-Cys with high sensitivity and selectivity. Moreover, the fluorescent probe was applied to detect tap water and well water with satisfactory results.
Starting Page	2093
Ending Page	2100
Page Count	8
File Format	HTM / HTML PDF
ISSN	20507526
Volume Number	3
Issue Number	9
Journal	Journal of Materials Chemistry C
DOI	10.1039/c4tc02394c
Language	English
Publisher	Royal Society of Chemistry
Access Restriction	Open
Subject Keyword	CNNS Fourier Graphitic carbon nitride Nitride Ultrasound Transmission electron microscopy Atomic-force microscopy X-ray scattering techniques X-ray crystallography Crystal structure Photoemission spectroscopy Fourier-transform infrared spectroscopy Fluorescence Quantum tunnelling Project Mercury Ion Covalent bond Cysteine Thiol
Content Type	Text
Resource Type	Article
Subject	Chemistry Materials Chemistry

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