NDLI: Preparation of hierarchical C@MoS<sub>2</sub>@C sandwiched hollow spheres for lithium ion batteries

Content Provider	Royal Society of Chemistry (RSC)
Author	Ottmann, Alexander Zhang, Ting Sun, Qing Vaynzof, Yana Meyer, Hans-Peter Xiang, Junhui Klingeler, Rüdiger Li, Zhenyou
Copyright Year	2017
Abstract	Hierarchical C@MoS2@C hollow spheres with active MoS2 nanosheets being sandwiched by carbon layers have been produced using a modified template method. The process applies polydopamine (PDA) layers that inhibit morphological changes of the template, enforcing the hollow microsphere structure. In addition, PDA forms complexes with the Mo precursor, leading to the in situ growth of MoS2 on its surface and preventing the nanosheets from agglomeration. It also supplies the carbon that finally sandwiches the 100–150 nm thin MoS2 spheres. The resulting hierarchically structured material provides a stable microstructure, where carbon layers strongly linked to MoS2 offer efficient pathways for electron and ion transfer, and concomitantly buffer the volume changes inevitably appearing during the charge–discharge process. Carbon-sandwiched MoS2-based electrodes exhibit high specific capacity of approximately 900 mA h g−1 after 50 cycles at 0.1C, excellent cycling stability up to 200 cycles, and superior rate performance. The versatile synthesis method reported here offers a general route to design hollow sandwich structures with a variety of different active materials.
Starting Page	3987
Ending Page	3994
Page Count	8
File Format	HTM / HTML PDF
ISSN	20507488
Volume Number	5
Issue Number	8
Journal	Journal of Materials Chemistry A
DOI	10.1039/c6ta10439h
Language	English
Publisher	Royal Society of Chemistry
Access Restriction	Open
Subject Keyword	Mo Carbon Personal digital assistant Microparticle Ion Sandwich compound
Content Type	Text
Resource Type	Article
Subject	Chemistry Renewable Energy, Sustainability and the Environment Materials Science

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