NDLI: Bridging chemical- and bio-catalysis: high-value liquid transportation fuel production from renewable agricultural residues

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Fluoride-free and low concentration template synthesis of hierarchical Sn-Beta zeolites: efficient catalysts for conversion of glucose to alkyl lactate

Acid promoted C–C bond oxidative cleavage of β-O-4 and β-1 lignin models to esters over a copper catalyst

An enolate ion as a synthon in biocatalytic synthesis of 3,4-dihydro-2(1H)-quinoxalinones and 3,4-dihydro-1,4-benzoxazin-2-ones: lemon juice as an alternative to hazardous solvents and catalysts

A nanoporous nickel catalyst for selective hydrogenation of carbonates into formic acid in water

5-Hydroxymethyl-2-vinylfuran: a biomass-based solvent-free adhesive

Recovery and esterification of aqueous carboxylates by using CO₂-expanded alcohols with anion exchange

PVP-Pd nanoparticles as efficient catalyst for nitroarene reduction under mild conditions in aqueous media

Unique nanocages of 12CaO·7Al₂O₃ boost heterolytic hydrogen activation and selective hydrogenation of heteroarenes over ruthenium catalyst

Co-Pyrolysis of torrefied biomass and methane over molybdenum modified bimetallic HZSM-5 catalyst for hydrocarbons production

Hierarchically nanostructured MnCo₂O₄ as active catalysts for the synthesis of N-benzylideneaniline from benzyl alcohol and aniline

Solid base catalyzed depolymerization of lignin into low molecular weight products

NHC-based coordination polymers as solid molecular catalysts for reductive amination of biomass levulinic acid

High quality sustainable Cu₂ZnSnSe₄ (CZTSe) absorber layers in highly efficient CZTSe solar cells

Potassium phosphate-catalyzed one-pot synthesis of 3-aryl-2-oxazolidinones from epoxides, amines, and atmospheric carbon dioxide

Highly chemoselective reduction of nitroarenes over non-noble metal nickel-molybdenum oxide catalysts

Superhydrophobic functionalization of cutinase activated poly(lactic acid) surfaces

Pd/C catalyzed phenoxycarbonylation using N-formylsaccharin as a CO surrogate in propylene carbonate, a sustainable solvent

An optimised synthesis of high performance radiation-grafted anion-exchange membranes

A photoactive catalyst Ru–g-C₃N₄ for hydrogen transfer reaction of aldehydes and ketones

Nitrate reduction on the surface of bimetallic catalysts supported by nano-crystalline beta-zeolite (NBeta)

Inside back cover

Back cover

Green Chemistry Vol - 19 Issue - 2

Green Chemistry Vol - 19 Issue - 1

Green Chemistry Vol -9

Green Chemistry Vol -8

Green Chemistry Vol -7

Green Chemistry Vol -6

Green Chemistry Vol -5

Green Chemistry Vol -4

Green Chemistry Vol -3

Green Chemistry Vol -2

Bridging chemical- and bio-catalysis: high-value liquid transportation fuel production from renewable agricultural residues

Content Provider	Royal Society of Chemistry (RSC)
Author	Liu, Fangfang Yang, Shang-Tian Guo, Xinwen Chen, Lijie Bai, Fengwu Hudson, Elton P. Xue, Chuang Liu, Min
Copyright Year	2017
Abstract	Catalytic conversion of lignocellulosic biomass to high-value transportation petrol, jet and diesel fuels is of great importance to develop versatile renewable energy and boost the rural economy, thus it is receiving worldwide attention. However, the state-of-the-art processes still suffer from a low efficiency in yield and productivity, which hinders the progress of its commercialization. Thus, it is essential to explore the consolidated catalytic reaction and refinery process. Here we report an advanced approach/process that could continuously produce long-chain (C5–C15) ketones from lignocellulosic biomass in a cascade mode by integrating several bio- and chemical catalysis reactions/processes, which exhibits a high efficiency and stable conversion rate. This technology consolidated the acetone–butanol–ethanol (ABE) fermentation, palladium catalyzed alkylation and in situ product recovery, allowing the catalytic reaction to proceed consistently and smoothly. The remarkable conversion properties are mainly attributed to the excellent compatible linkage of chemical catalysis with biosynthesis and process design to stabilize the Pd catalytic reaction. This validated strategy for the rational process design and integration of chemical- and bio-catalysis offers great demonstration in producing high-value transportation biofuels derived from agricultural residues.
Starting Page	660
Ending Page	669
Page Count	10
File Format	HTM / HTML PDF
ISSN	14639262
Volume Number	19
Issue Number	3
Journal	Green Chemistry
DOI	10.1039/c6gc02546c
Language	English
Publisher	Royal Society of Chemistry
Access Restriction	Open
Subject Keyword	Lignocellulosic biomass Renewable resource Fermentation
Content Type	Text
Resource Type	Article
Subject	Environmental Chemistry Pollution

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1	Ministry of Education (GoI), Department of Higher Education	Sanctioning Authority	https://www.education.gov.in/ict-initiatives
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3	National Digital Library of India Office, Indian Institute of Technology Kharagpur	The administrative and infrastructural headquarters of the project	Dr. B. Sutradhar bsutra@ndl.gov.in
4	Project PI / Joint PI	Principal Investigator and Joint Principal Investigators of the project	Dr. B. Sutradhar bsutra@ndl.gov.in Prof. Saswat Chakrabarti will be added soon
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