NDLI: Hydrogen photogeneration from water on the biomimetic hybrid artificial photocatalytic systems of semiconductors and earth-abundant metal complexes: progress and challenges

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Hydrogen photogeneration from water on the biomimetic hybrid artificial photocatalytic systems of semiconductors and earth-abundant metal complexes: progress and challenges

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Catalysis Science & Technology Vol - 5 Issue - 5

Catalysis Science & Technology Vol - 5 Issue - 4

Catalysis Science & Technology Vol - 5 Issue - 3

Catalysis Science & Technology Vol - 5 Issue - 2

Catalysis Science & Technology Vol -4

Catalysis Science & Technology Vol -3

Catalysis Science & Technology Vol -2

Catalysis Science & Technology Vol -1

Hydrogen photogeneration from water on the biomimetic hybrid artificial photocatalytic systems of semiconductors and earth-abundant metal complexes: progress and challenges

Content Provider	Royal Society of Chemistry (RSC)
Author	Xu, You Zhang, Bin
Copyright Year	2015
Abstract	The replacement of traditional non-renewable fossil fuels by sustainable energy sources is one of the most challenging problems that must be solved in the 21st century. In this context, the conversion of solar energy into stored chemical energy, especially the solar-driven splitting of water into molecular H2 and O2, has emerged as an attractive technology to solve the global energy issue. Inspired, but not constrained, by natural photosynthesis, a number of artificial systems and devices have been developed to harvest sunlight, oxidise water and reduce protons to produce useful solar fuels. This perspective reviews the recent significant developments in the field of hybrid artificial photocatalytic systems containing semiconductors as the photosensitizer, and organometallic complexes made of earth-abundant elements (Fe, Co, Ni) as the molecular catalyst, for the photogeneration of H2 from water. A brief introduction to artificial photosynthesis and water reduction is first given, followed by an explanation of the basic principles and mechanism involved in artificial solar-driven water splitting for H2 generation. Different series of hybrid artificial photocatalytic systems based on semiconductor photosensitizers and molecular catalysts that can be applied in the photogeneration of H2 from water are discussed in detail. Finally, the future perspectives of this research field are also discussed.
Starting Page	3084
Ending Page	3096
Page Count	13
File Format	HTM / HTML PDF
ISSN	20444753
Volume Number	5
Issue Number	6
Journal	Catalysis Science & Technology
DOI	10.1039/c5cy00365b
Language	English
Publisher	Royal Society of Chemistry
Access Restriction	Open
Subject Keyword	Oxygen Water splitting Semiconductor Organometallic chemistry Solar energy Artificial photosynthesis Fossil fuel Photosynthesis Sustainable energy Photosensitizer
Content Type	Text
Resource Type	Article
Subject	Catalysis

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