NDLI: A review of high temperature co-electrolysis of H<sub>2</sub>O and CO<sub>2</sub> to produce sustainable fuels using solid oxide electrolysis cells (SOECs): advanced materials and technology

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A review of high temperature co-electrolysis of H₂O and CO₂ to produce sustainable fuels using solid oxide electrolysis cells (SOECs): advanced materials and technology

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Chemical Society Reviews Vol - 46 Issue - 4

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A review of high temperature co-electrolysis of H₂O and CO₂ to produce sustainable fuels using solid oxide electrolysis cells (SOECs): advanced materials and technology

Content Provider	Royal Society of Chemistry (RSC)
Author	Zhang, Wenqiang Wang, Jianchen Zhang, Jiujun Yu, Bo Zheng, Yun Chen, Jing Qiao, Jinli
Copyright Year	2017
Abstract	High-temperature solid oxide electrolysis cells (SOECs) are advanced electrochemical energy storage and conversion devices with high conversion/energy efficiencies. They offer attractive high-temperature co-electrolysis routes that reduce extra CO2 emissions, enable large-scale energy storage/conversion and facilitate the integration of renewable energies into the electric grid. Exciting new research has focused on CO2 electrochemical activation/conversion through a co-electrolysis process based on the assumption that difficult CO double bonds can be activated effectively through this electrochemical method. Based on existing investigations, this paper puts forth a comprehensive overview of recent and past developments in co-electrolysis with SOECs for CO2 conversion and utilization. Here, we discuss in detail the approaches of CO2 conversion, the developmental history, the basic principles, the economic feasibility of CO2/H2O co-electrolysis, and the diverse range of fuel electrodes as well as oxygen electrode materials. SOEC performance measurements, characterization and simulations are classified and presented in this paper. SOEC cell and stack designs, fabrications and scale-ups are also summarized and described. In particular, insights into CO2 electrochemical conversions, solid oxide cell material behaviors and degradation mechanisms are highlighted to obtain a better understanding of the high temperature electrolysis process in SOECs. Proposed research directions are also outlined to provide guidelines for future research.
Starting Page	1427
Ending Page	1463
Page Count	37
File Format	HTM / HTML PDF
ISSN	03060012
Volume Number	46
Issue Number	5
Journal	Chemical Society Reviews
DOI	10.1039/c6cs00403b
Language	English
Publisher	Royal Society of Chemistry
Access Restriction	Open
Subject Keyword	Water High-temperature electrolysis Oxygen Electrode Renewable energy Electrochemistry Solid oxide electrolyser cell SOEC
Content Type	Text
Resource Type	Article
Subject	Chemistry

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