NDLI: Insight on Reaction Pathways of Photocatalytic CO<sub>2</sub> Conversion.

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Insight on Reaction Pathways of Photocatalytic CO₂ Conversion.

Content Provider	Europe PMC
Author	Wang, Yiou Chen, Enqi Tang, Junwang
Copyright Year	2022
Abstract	Photocatalytic CO2 conversion to value-added chemicalsis a promising solution to mitigate the current energy and environmentalissues but is a challenging process. The main obstacles include theinertness of CO2 molecule, the sluggish multi-electronprocess, the unfavorable thermodynamics, and the selectivity controlto preferable products. Furthermore, the lack of fundamental understandingof the reaction pathways accounts for the very moderate performancein the field. Therefore, in this Perspective, we attempt to discussthe possible reaction mechanisms toward all C1 and C2 value-added products, taking into account the experimentalevidence and theoretical calculation on the surface adsorption, protonand electron transfer, and products desorption. Finally, the remainingchallenges in the field, including mechanistic understanding, reactordesign, economic consideration, and potential solutions, are criticallydiscussed by us.
Related Links	https://europepmc.org/backend/ptpmcrender.fcgi?accid=PMC9207809&blobtype=pdf
Journal	ACS Catalysis [ACS Catal]
Volume Number	12
DOI	10.1021/acscatal.2c01012
PubMed Central reference number	PMC9207809
Issue Number	12
PubMed reference number	35747201
e-ISSN	21555435
Language	English
Publisher	American Chemical Society
Publisher Date	2022-06-03
Access Restriction	Open
Rights License	Permits the broadest form of re-use including for commercial purposes, provided that author attribution and integrity are maintained (https://creativecommons.org/licenses/by/4.0/). © 2022 The Authors. Published by American Chemical Society
Subject Keyword	CO2 conversion photocatalysis mechanism reaction pathways selectivity
Content Type	Text
Resource Type	Article
Subject	Chemistry Catalysis

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4	Project PI / Joint PI	Principal Investigator and Joint Principal Investigators of the project	Dr. B. Sutradhar bsutra@ndl.gov.in Prof. Saswat Chakrabarti will be added soon
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