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High-performance perovskite CH3NH3PbI3 thin films for solar cells prepared by single-source physical vapour deposition.
| Content Provider | Europe PMC |
|---|---|
| Author | Fan, Ping Gu, Di Liang, Guang-Xing Luo, Jing-Ting Chen, Ju-Long Zheng, Zhuang-Hao Zhang, Dong-Ping |
| Copyright Year | 2016 |
| Abstract | In this work, an alternative route to fabricating high-quality CH3NH3PbI3 thin films is proposed. Single-source physical vapour deposition (SSPVD) without a post-heat-treating process was used to prepare CH3NH3PbI3 thin films at room temperature. This new process enabled complete surface coverage and moisture stability in a non-vacuum solution. Moreover, the challenges of simultaneously controlling evaporation processes of the organic and inorganic sources via dual-source vapour evaporation and the heating process required to obtain high crystallization were avoided. Excellent composition with stoichiometry transferred from the powder material, a high level of tetragonal phase-purity, full surface coverage, well-defined grain structure, high crystallization and reproducibility were obtained. A PCE of approximately 10.90% was obtained with a device based on SSPVD CH3NH3PbI3. These initial results suggest that SSPVD is a promising method to significantly optimize perovskite CH3NH3PbI3 solar cell efficiency. |
| Journal | Scientific Reports [Sci Rep] |
| Volume Number | 6 |
| DOI | 10.1038/srep29910 |
| PubMed Central reference number | PMC4947921 |
| PubMed reference number | 27426686 |
| e-ISSN | 20452322 |
| Language | English |
| Publisher | Nature Publishing Group |
| Publisher Date | 2016-07-18 |
| Access Restriction | Open |
| Content Type | Text |
| Resource Type | Article |
| Subject | Multidisciplinary |