NDLI: Capture and conversion of CO2 at ambient conditions by a conjugated microporous polymer.

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Capture and conversion of CO2 at ambient conditions by a conjugated microporous polymer.

Content Provider	Europe PMC
Author	Xie, Yong Wang, Ting-Ting Liu, Xiao-Huan Zou, Kun Deng, Wei-Qiao
Copyright Year	2013
Abstract	Conjugated microporous polymers are a new class of porous materials with an extended π-conjugation in an amorphous organic framework. Owing to the wide-ranging flexibility in the choice and design of components and the available control of pore parameters, these polymers can be tailored for use in various applications, such as gas storage, electronics and catalysis. Here we report a class of cobalt/aluminium-coordinated conjugated microporous polymers that exhibit outstanding CO2 capture and conversion performance at atmospheric pressure and room temperature. These polymers can store CO2 with adsorption capacities comparable to metal-organic frameworks. The cobalt-coordinated conjugated microporous polymers can also simultaneously function as heterogeneous catalysts for the reaction of CO2 and propylene oxide at atmospheric pressure and room temperature, wherein the polymers demonstrate better efficiency than a homogeneous salen-cobalt catalyst. By combining the functions of gas storage and catalysts, this strategy provides a direction for cost-effective CO2 reduction processes.
Journal	Nature Communications [Nat Commun]
Volume Number	4
DOI	10.1038/ncomms2960
PubMed Central reference number	PMC3709476
PubMed reference number	23727768
e-ISSN	20411723
Language	English
Publisher	Nature Publishing Group
Publisher Date	2013-01-01
Access Restriction	Open
Content Type	Text
Resource Type	Article
Subject	Chemistry Biochemistry, Genetics and Molecular Biology Physics and Astronomy

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